Whe unpredictable is used negatively it usually mean being unclear about exceptations.
Say Bob wants to make Alice happy and therefore buys her jewellery. Afterwards Alice complains that Bob is to materalistic and that money gets better spend on helping starving children in Africa.
If Bob can't predict such a response from Alice after a while of being together with her he would probablly call her unpredicable in a negative way.
You should be clear about the kind of how you expect to be treated from other people.
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